CALIBURN: Self-Calibrated LLM Unlearning Alignment

Large language models (LLMs) trained on unfiltered corpora inherently risk retaining sensitive information, necessitating selective knowledge unlearning for regulatory compliance and ethical safety. However, existing parameter-modifying methods face fundamental limitations: high computational costs, uncontrollable forgetting boundaries, and strict dependency on model weight access. These constraints render them impractical for closed-source models, yet current non-invasive alternatives remain unsystematic and reliant on empirical experience. To address these challenges, we propose the Controllable Alignment Prompting for Unlearning (CAP) framework, an end-to-end prompt-driven unlearning paradigm. CAP decouples unlearning into a learnable prompt optimization process via reinforcement learning, where a prompt generator collaborates with the LLM to suppress target knowledge while preserving general capabilities selectively. This approach enables reversible knowledge restoration through prompt revocation. Extensive experiments demonstrate that CAP achieves precise, controllable unlearning without updating model parameters, establishing a dynamic alignment mechanism that overcomes the transferability limitations of prior methods.

Machine unlearning for large language models (LLMs) aims to selectively remove memorized content such as private data, copyrighted text, or hazardous knowledge, without costly full retraining. Most existing methods require a retain set of curated examples to prevent catastrophic degradation of general model utility, creating an extra data dependency that complicates deployment. We propose SHRED (Self-distillation via High-surprisal-only Retain-set-free Entropy Demotion), a retain-set-free unlearning method built on a key insight: not all tokens within a forget set instance carry memorized information equally. High-information tokens concentrate the model's memorized knowledge, while low-information tokens reflect general language competence. SHRED operates in two stages. (1) Selection: We perform a forward pass on a forget set instance, collect per-token autoregressive probabilities, and select the bottom (lowest probability, highest Shannon information) as forget positions; the remaining positions are retained as benign anchors. (2) Training: We construct modified KL targets that demote the memorized token's logit at forget positions while preserving the original distribution at benign positions. The model is then trained via a single top KL self-distillation objective that simultaneously drives forgetting and utility preservation. We evaluate SHRED across four standard unlearning benchmarks and demonstrate that it establishes a new Pareto-optimal trade-off between forget efficacy and model utility, outperforming retain-set-dependent methods. Our analysis shows that SHRED is robust against relearning attacks and membership-inference attacks, and it maintains stable utility even after many sequential unlearning runs.

Mitigating sensitive and harmful outputs is fundamental to ensuring safe deployment of LLMs. Existing approaches typically follow two paradigms: Knowledge Deletion (KD), which erases undesirable information during training, and Distinguishable Refusal (DR), which steers models away from using sensitive knowledge during inference. Despite rapid progress, KD-based unlearning struggles with biased deletion due to suppressing specific token sequences as a substitute for complete knowledge removal, whereas DR-based unlearning risks the re-emergence of harmful knowledge because the underlying knowledge remains intact. To address these issues, we propose Distinguishable Deletion ($\mathrm{D^2}$), a paradigm that restricts the response distribution in the latent representation rather than specific tokens to erase undesirable knowledge, while distinguishing it from retained knowledge, enabling a refusal mechanism to handle unlearned inputs safely and coherently. To implement $\mathrm{D^2}$, we introduce an energy index that quantifies the presence of knowledge and the separation between unlearned and retained content. Mathematical and empirical analyses show that energy is both accurate and efficient, enabling Energy-based Unlearning Alignment (EUA) to enforce energy-boundary unlearning during training and apply an energy-based refusal mechanism at inference. Extensive experiments demonstrate that EUA significantly outperforms previous methods, indicating the superiority of $\mathrm{D^2}$. Our code is available at https://github.com/Puning97/EUA-for-LLM-Unlearning.