Do large language models' (LLMs') answers to self-report questionnaires predict how they behave? Prior work finds they do not, but it uses human personality inventories, so the gap could reflect borrowed human constructs rather than LLM self-report itself. We test this with a self-report instrument built from LLM-specific behaviors (e.g., over-refusal, unsolicited disclaimers) whose structure is derived bottom-up. Administering 300 items 30 times to 25 LLMs from 17 developers yields five replicable, reliable factors (Tucker
φ≥.957,
α≥.930). We compare these self-reports with 2,500 open-ended behavioral samples rated by 151 humans and an LLM-judge ensemble. Humans and judges agree about model behavior (
rˉ=.51), but self-report barely tracks human ratings (
rˉ=.09, 95% CI
[−.07,.18]) or rater-free text measures, and correcting for criterion unreliability leaves four of five factors near zero. Verbosity is the partial exception (
r=.40, 71% of its reliability ceiling). On Responsiveness, self-report tracks LLM judges more than humans (
r=.53 vs.
.18; Steiger
p=.04), and controlling for length and formatting does not remove this: agreement between LLM judges and LLM self-report is weak evidence that either tracks human judgment.