Air Quality Prediction

Nitrogen dioxide (NO2) is a common air pollutant, released into the atmosphere through the incomplete burning of fossil fuels, and associated with respiratory and cardiovascular diseases in humans. Ambient NO2 concentrations are regulated through air-quality limits assessed with a sparse network of fixed monitors. The revised EU Ambient Air Quality Directive (2024/2881) introduces a daily NO2 limit to be met from 2030. At present, neither the regulatory monitoring network nor existing coarse, annual-mean models can resolve NO2 concentrations at the spatio-temporal resolutions necessary to assess compliance. Here we map NO2 across Europe at hourly and 10m resolution with a machine-learning model that combines ground monitors with satellite, reanalysis, land-use, traffic and emission data and returns a calibrated predictive distribution at every location. Validated against held-out regulatory monitors and independent citizen-science campaigns, the maps resolve high-resolution spatiotemporal NO2 gradients for 110 metropolitan areas in Europe. We reconstruct the daily compliance statistic across those regions and find limit breaches in 91 EU air quality zones deemed compliant by the regulatory monitoring network, covering a population of approximately 135M. Beyond air quality zones and monitor locations, an estimated 9-9.4% (20M) of the population in mapped regions lives in areas where the daily NO2 limit is breached. The high-resolution maps offer a route to population-scale assessment of compliance with the 2030 limits.

Urban air quality can vary significantly along transit corridors, necessitating high-resolution monitoring. This work introduces a novel mobile-sensing dataset from Surat, Gujarat, India, comprising PM$*{2.5}$ concentrations, meteorological variables (temperature, humidity, wind speed, wind direction), and land-use features. To represent the spatiotemporal data as a graph, two node-definition strategies were used: (i) uniform segmentation (200--400~m intervals) and (ii) DBSCAN clustering to adaptively group dense observations. For each node, rolling mean and standard deviation of meteorological variables were computed. To model this high-dimensional data, we propose a SA-GNN for fine-grained, short-term PM$*{2.5}$ forecasting and hotspot identification. We compared SA-GNN with LSTM, RNN, GRU, and ANN models. These models performed well on low-resolution data but had difficulty capturing rapidly changing patterns in urban air quality. SA-GNN employs cluster-specific GRUs to capture localized temporal dependencies and a Graph Attention Network to learn spatial heterogeneity. This hybrid architecture effectively models rapid fluctuations and complex spatial interactions. On our dataset, SA-GNN achieved $R^2 = 0.95$, RMSE $= 6.8$, and MAE $= 4.2~\si{\micro\gram\per\meter\cubed}$, outperforming all baseline models. Combining spatial clustering with adaptive attention significantly improves forecasting, enabling real-time, fine-grained monitoring and supporting personalized exposure tracking and timely alerts for healthier cities.

Which meteorological processes control exposure to fugitive gases downwind of a source, and on what timescales, have largely been inferred from dispersion theory and partial field evidence. Here we show that the meteorological drivers of elevated hydrogen sulphide (H$_2$S) exposure at a long-monitored European landfill, and the timescales over which each acts, can be identified directly from monitoring data. Wind direction, wind speed and atmospheric pressure form the causal core, with the share of directed information carried by pressure increasing with aggregation scale. The recovered timescales are consistent with those expected from the underlying atmospheric processes. We use these driver timescales to initialise CAIRN (Causal-Anchored Inference for Receptor Nowcasting), a machine-learning nowcaster with fast and slow memory components. Trained on past exceedances of WHO guideline levels, CAIRN nowcasts them from surface weather measurements and the calendar alone, without hand-engineered features. Combining four such nowcasters produces a site-level, tiered alert that agrees substantially with that generated by a direct sensor network and tracks an independent record of community odour reports. Meteorological variables can therefore serve as an inference-time proxy for exposure relative to WHO guideline levels, and they link atmospheric dynamics to community impact as an episode unfolds.

Poor air quality in urban areas is driven by a complex chain of processes and presents a significant public health concern. To better understand and control the mechanisms that determine air quality, cities deploy networks of measurement stations, and launch initiatives for collecting denser data about the concentration of pollutants in the atmosphere. Extracting insights from the stations relies on their reliable and uninterrupted operation. However, hardware is susceptible to faults and black- outs that may result in data unavailability, which affects the overall quality of analyses. In this paper, we present a deep-learning model, called SATADL, which can infer complex relations and output multiple-hour-ahead air-quality forecasts. The goal of the model is to simulate the mea- surements of an unresponsive station until its operation is restored. The architecture of the model, which allows it to extract information from different aspects of the data, is described in detail and a careful examination of all of its components is provided. We demonstrate the performance of SATADL on four sets of air quality stations from around the world, by using it to simulate the concentration of PM10 for periods of hypothetical failures of one of the measurement stations, lasting for as long as 48 hours. A selection of baseline and published deep learning models were trained and used as a benchmark. The results show that SATADL per- forms better across different prediction windows, for both coefficient of determination and root mean squared error, demonstrating its suitability as a virtual proxy station.

Accurate air quality forecasting is essential for public health and urban environmental management, but remains challenging because pollutant channels differ in periodicity and distribution drift, while their concentration trajectories contain both multi-scale dependencies and rapid changes. Recent methods have improved spatial dependency learning and meteorological covariate modeling. However, pollutant channels are still passed through the same normalization rule and temporal backbone, using a shared latent representation for channel-specific distributions and changes at different rates. To address this limitation, we propose AirFlow, a pollutant-aware dual-stream framework that operates on station multivariate observations without additional graph propagation or predefined signal decomposition. Specifically, AirFlow designs two novel blocks: (1) a statistic-guided normalization routing mechanism that selects a normalization path for each pollutant according to its 24-hour autocorrelation and distribution drift; and (2) a hierarchical dual-stream state model that combines multi-scale state space propagation with learnable response coefficients, where gated bidirectional cross-attention exchanges information and adaptively fuses the resulting representations. Experiments on real-world data from multiple cities show that AirFlow achieves the best performance in 34 of 36 metrics comparisons, with reductions of up to 11.11% root mean square error over the state-of-the-art baseline. AirFlow also requires only 0.0483M parameters and 0.0215G FLOPs, achieving high forecasting accuracy with low computational overhead.

Weather forecasting foundation models (FMs) are increasingly fine-tuned to predict air quality, offering fast global pollution forecasts at lower computational cost than conventional chemical transport models. These FMs are typically trained on reanalysis data and generate forecasts through autoregressive rollout. They do not explicitly represent governing physical or chemical processes. Therefore, high forecast skill does not reveal whether a model has learned physical mechanisms or exploits statistical regularities in its training data. Here, we present the first study of what a FM fine-tuned for atmospheric chemistry has learned by examining Microsoft's Aurora model. We impose controlled chemical perturbations on its forecasts and test them against known photochemical relationships. We then examine the internal representations that generate these forecasts. We find that Aurora captures a first-order ozone response to reactive nitrogen but does not enforce the chemical constraints that a process-based model encodes. It generates chemically inconsistent combinations of related species and relaxes localized emission features such as wildfire plumes toward background. Internally, its representations remain largely organized around the meteorology inherited during pretraining, with little structure specific to chemistry. Using sparse autoencoders, we identify internal components that causally control the chemical forecast but do not map cleanly onto individual atmospheric processes. This work provides a framework for testing whether AI forecasting systems learn atmospheric chemistry from reanalysis data. As these models are increasingly positioned to inform environmental policy decisions, we argue that composition forecasts should also be judged by their internal mechanisms rather than by benchmark skill alone.

Air pollution and climate-related stressors are increasingly important concerns for respiratory health, especially in settings with unequal environmental exposure and healthcare capacity. This study evaluates an interpretable machine learning framework for predicting respiratory disease rates and air-quality status using structured country-level weekly data. Two supervised learning tasks were considered: regression of respiratory disease rate per 100,000 population and binary classification of air-quality status. Nine regression models and nine classification models were compared using nested cross-validation. Model interpretation was conducted using SHAP values, and subgroup analysis was performed across income levels and geographic regions. The results showed that PM2.5 concentration was the dominant predictor of respiratory disease rate, with linear and regularized linear models achieving the strongest regression performance. For air-quality classification, models achieved high balanced accuracy when PM2.5 was included, but performance decreased substantially when PM2.5 was removed, indicating strong dependence on pollutant-related information. SHAP analysis showed that, without PM2.5, socioeconomic and meteorological variables such as GDP per capita, precipitation, and healthcare access became more influential. Subgroup analysis showed similar aggregate regression error across income groups, but PM2.5 contributed more strongly to predictions in lower-middle-income countries. These results show that model accuracy alone is not sufficient for climate-health prediction. Interpretable models can help identify dominant pollution-related signals, test whether results depend on key pollutant variables, and show whether prediction patterns differ across socioeconomic groups.

Wildfire smoke events produce extreme PM$_{2.5}$ concentrations that pose severe public health risks, yet forecasting rare, hazardous-level spikes remains a fundamental challenge. Time series foundation models (TSFMs), pretrained models offering zero-shot inference and efficient adaptation, perform strongly on general benchmarks, but their behavior under extreme out-of-distribution conditions is poorly understood. We present the first systematic benchmark comparing six TSFM configurations (zero-shot TimesFM, Chronos-2, Moirai-2, and Time-MoE, plus LoRA fine-tuned Chronos-2 and Time-MoE) against fully-trained baselines (LSTM, BiLSTM, Transformer) and naive persistence on a 12-year (2013--2025) hourly PM$_{2.5}$ dataset covering 1,375 wildfire incidents across 79 California monitoring sites. A leave-one-incident-out (LOIO) protocol evaluates generalization to unseen fires, using MAE, RMSE, and exceedance F1 at EPA AQI thresholds across 6-, 12-, and 24-hour horizons. Results reveal a consistent hierarchy. The BiLSTM achieves the lowest MAE ($5.16\,μg/m^3$) and the highest exceedance F1 at every threshold, including the Hazardous band ($>225.5\,μg/m^3$), reaching 0.63 versus at most 0.54 for any foundation model. Zero-shot TSFMs improve on persistence only modestly, and zero-shot Chronos-2 exhibits severe RMSE tail instability ($23.4\,μg/m^3$, negative $R^2$) from sporadic large errors. LoRA fine-tuning substantially improves both adapted families and largely repairs this instability, yet no foundation model surpasses the trained recurrent baselines on any metric. These findings challenge the assumption that larger pretrained models universally dominate environmental forecasting and provide actionable deployment guidance for wildfire air quality prediction.

Super-resolving coarse atmospheric fields to local PM$_{2.5}$ variations is uniquely challenged by a mismatch in spatial support: while pixels represent regional averages, ground-truth observations are discrete, unaligned samples of a continuous spatial signal. To bridge this gap, we present a station-guided framework for high-resolution PM$_{2.5}$ downscaling over Europe. Taking coarse CAMS atmospheric composition fields alongside heterogeneous side information (i.e., human activity, land cover, elevation, satellite aerosol observations, and wind fields) our framework jointly super-resolves ($\times 40$, $\approx$ 1 km) and bias-corrects CAMS rasters, without relying on temporal sequence modelling. To address the challenge of densely supervising our multi-scale transformer network with sparse in-situ data, we introduce a time-agnostic propagation strategy that utilises spatial Gaussian blending of interpolated OpenAQ observations. Extensive qualitative and station-level evaluations across Europe demonstrate that our model recovers fine-grained spatial structures and effectively mitigates localised CAMS biases.

Accurate particulate matter (PM) prediction is crucial for mitigating air pollution. Graph Neural Networks (GNNs) effectively model spatiotemporal dependencies, but predefined graphs limit adaptability, and some datasets complicate learning. This study introduces a graph construction method based on a confusion matrix from a supervised learning process to dynamically capture inter-class relationships. Additionally, a hybrid loss function that combines energy distance and Huber loss is applied to address the vanishing gradient problem and improve learning stability. The approach is evaluated using air pollution data from the University of Utah AirU Pollution Monitoring Network in Salt Lake City, UT, with five GNN models: Graph Convolutional Networks (GCNs), Simple Graph Convolutional Networks (SGConv), Graph Isomorphism Networks (GINs), Graph Attention Networks (GATs), and GraphSage. The experimental results of single- and multistep predictions confirm that GraphSage achieves the highest accuracy in predicting the concentrations of PM${1}$, PM${10}$, and PM$_{2.5}$ over different time horizons. Furthermore, {\color{black} GNNExplainer (Graph Neural Network Explainer) and PGExplainer (Probabilistic Graph Explainer)} are applied to interpret feature importance and graph structure, ensuring model transparency. Results show improved prediction accuracy, with GNN models outperforming traditional machine learning \textcolor{black}{and deep learning models (i.e., Prophet, Long short-term memory, Gated recurrent units} in air pollution forecasting.

Accurate short-term PM$_{2.5}$ forecasting is important for public health protection, air-quality early warning, and urban environmental management. However, PM$_{2.5}$ variation is driven by multiple coupled factors, including stable periodic changes induced by human activities and meteorological regularity, station-specific short-term concentration evolution, and meteorology-driven pollutant dispersion among monitoring stations. Existing spatio-temporal forecasting methods may capture station relationships to some extent, but distance-only, correlation-based, or purely adaptive graphs are often insufficient to comprehensively represent these heterogeneous factors, especially wind-direction-dependent pollutant transport. To address this problem, we propose a Multi-View Geo-Wind Guided KAN model for PM$_{2.5}$ forecasting, named \textbf{MVG-KAN}, which models station-level PM$_{2.5}$ evolution from three complementary views: local periodic regularity, station-wise residual temporal dynamics, and meteorological-environment-guided spatial dispersion. Specifically, the periodic-residual forecasting backbone first separates stable daily and weekly patterns from non-periodic residual variations. A Geo-Wind Graph is constructed by combining geographic distance decay with wind-direction- and wind-speed-aware transport, providing a lightweight physically motivated directed spatial prior for residual propagation among stations. In addition, a temporal Kolmogorov-Arnold network (TKAN) residual head is then introduced to learn station-wise nonlinear autoregressive correction from de-periodized PM$_{2.5}$ residuals and historical multi-pollutant sequences, thereby enhancing the modeling of local residual inertia and pollutant co-variation.

Forecasting particulate matter (PM10) requires both station-scale accuracy and continuous spatial fields, especially during severe dust storms. Chemical transport models (CTMs) provide gridded forecasts but retain local biases, whereas graph neural networks (GNNs) track monitoring sites well at short lead times but do not produce gridded outputs. Here we present OmniPM-Net, a Convolutional Conditional Neural Process (ConvCNP)-based fusion model that reconciles these two forecast types within a shared spatial representation. A terrain-aware Gaussian set convolution lifts irregular GNN station forecasts onto a regular grid, where a multi-scale Spatial Source Attention (SSA) module blends them with Copernicus Atmosphere Monitoring Service (CAMS) forecasts; a shared omni-query readout then decodes this representation into consistent PM10 predictions at either stations or grid cells over a 108 h horizon. Evaluated across 1,618 air-quality monitoring stations throughout China over the full year of 2024, OmniPM-Net matches the station-level accuracy of the stronger GNN baseline (mean absolute error 21.14 versus 22.00 ug/m3) and reduces the CAMS mean absolute error by 30%, while simultaneously delivering the gridded fields that the discrete GNN cannot. Its clearest gains are in the high-concentration tail, where the 90th-percentile MAE falls by 9% relative to the GNN and 25% relative to CAMS, and during dust episodes, where it improves categorical detection skill while tracking the evolving spatial trajectory.

Air pollution represents one of the most critical environmental and public health challenges globally, with traditional sensor-based monitoring systems facing significant scalability and economic constraints. Image-based air quality estimation has emerged as a promising alternative, leveraging the visual characteristics of atmospheric pollutants in traffic scenes. However, existing methods suffer from limited cross-city generalization and inadequate exploitation of multi-view perspectives. We present AQIFormer, a novel transformer-based ensemble architecture that addresses these fundamental limitations through innovative dual-view integration, weather-aware attention mechanisms, and comprehensive multi-task learning. Our approach uniquely combines front and rear traffic imagery with meteorological parameters to achieve robust air quality classification across diverse urban environments. Extensive evaluation on a comprehensive dataset of 26,678 synchronized front-rear image pairs demonstrates good performance with 89.96% accuracy, representing a 14.96% improvement over state-of-the-art methods. Most importantly, our model maintains exceptional cross-city generalization capabilities, achieving 81.67% accuracy on an independent dataset collected in Nagpur, India with only 8.29% performance degradation using few-shot adaptation with minimal training samples.

Accurate air quality prediction is essential for public health, environmental monitoring, and industrial safety. However, most existing approaches rely on centralized learning paradigms, which introduce challenges related to scalability, privacy preservation, and communication overhead in distributed Internet of Things (IoT) environments. Moreover, current federated learning (FL) based solutions predominantly utilize unimodal data, limiting their capability to capture complex environmental patterns. To address these limitations, we propose M$^2$FedAQI, a lightweight multimodal federated framework for decentralized Air Quality Index (AQI) prediction across heterogeneous edge devices. The proposed framework integrates visual and tabular modalities through a feature modulation based fusion mechanism that enables efficient cross-modal interaction while maintaining low computational overhead. M$^2$FedAQI is evaluated on two benchmark datasets, PM25Vision and TRAQID, for both classification and regression tasks under centralized and federated settings. Experimental results demonstrate that M$^2$FedAQI consistently outperforms existing approaches, achieving improvements of up to 11.0% in Accuracy, 3.53% in AUC, 12.2% in F1-score, and 18.0% in $R^2$, while reducing MAE and RMSE by up to 25.4% and 20.4%, respectively, compared with the strongest baselines. Furthermore, deployment on heterogeneous edge devices demonstrates efficient resource utilization in terms of communication overhead, memory footprint, and computational cost. To enhance communication security, TLS-based authentication is incorporated to ensure secure client participation and protect the FL communication channel from unauthorized third-party access without modifying the underlying FL protocol.

Air-quality forecasting models are commonly evaluated on regional, preprocessed, and normalized datasets, where missing observations are removed or artificially completed. Such protocols simplify comparison but hide the conditions that dominate real monitoring networks: uneven global coverage, structured missingness, heterogeneous pollutant scales, and deployment cost. We introduce \textbf{AirQualityBench}, a global multi-pollutant benchmark designed to evaluate forecasting models under these realistic conditions. The benchmark contains hourly observations from 3,720 monitoring stations over 2021--2025, covers six major pollutants, and preserves provider-native observation masks. Rather than imputing a dense data tensor, AirQualityBench exposes missingness as part of the forecasting problem and reports errors on valid future observations after inverse transformation to physical concentration scales. Evaluating representative spatio-temporal models under this unified protocol shows that strong performance on sanitized datasets does not reliably transfer to global, fragmented monitoring streams. AirQualityBench therefore serves as a realistic testbed for scalable, mask-aware, and physically interpretable air-quality forecasting. All benchmark data, code, evaluation scripts, and baseline implementations are available at GitHub.

Urban air quality forecasting is challenging because pollutant concentrations are nonlinear, nonstationary, spatiotemporally dependent, and often affected by anomalous observations caused by traffic congestion, industrial emissions, and seasonal meteorological variability. This study proposes a Graph Convolutional Support Vector Regression (GraphSVR) framework for robust spatiotemporal forecasting of urban air pollution. The model combines graph convolutional learning to capture inter-station spatial dependence with support vector regression to model nonlinear temporal dynamics while reducing sensitivity to outlier observations. The proposed framework is evaluated using air quality records from 37 monitoring stations in Delhi and 18 stations in Mumbai, representing inland and coastal metropolitan environments in India. Forecasting performance is assessed across multiple horizons and compared with established temporal and spatiotemporal benchmarks. The results show that GraphSVR consistently improves predictive accuracy and maintains stable performance across seasons and outlier-prone pollution episodes. Statistical test further confirms the reliability of the proposed approach across the datasets. Furthermore, the conformal prediction approach is integrated with GraphSVR to generate calibrated prediction intervals, enhancing its practical value for uncertainty-aware air quality monitoring and public health decision-making.

In this paper, we propose a Physics-Informed Neural Network framework for time-dependent simulations of pollution propagation originating from moving emission sources. We formulate a robust variational framework for the time-dependent advection-diffusion problem and establish the boundedness and inf-sup stability of the corresponding discrete weak formulation. Based on this mathematical foundation, we construct a robust loss function that is directly related to the true approximation error, defined as the difference between the neural network approximation and the (unknown) exact solution. Additionally, a collocation-based strategy is introduced to speed up neural network training. As a case study, we investigate pollution propagation caused by snowmobile traffic in Longyearbyen, Spitsbergen, supported by detailed in-field measurements collected using dedicated sensors. The proposed framework is applied to analyze the effects of thermal inversion on pollutant accumulation. Our results demonstrate that thermal inversion traps dense and humid air masses near the ground, significantly enhancing particulate matter (PM) concentration and worsening local air quality.

Air pollution is a worldwide public health threat that can cause or exacerbate many illnesses, including respiratory disease, cardiovascular disease, and some cancers. However, epidemiological studies and public health decision-making are stymied by the inability to assess pollution exposure impacts in near real time. To address this, developing accurate digital twins of environmental pollutants will enable timely data-driven analytics - a crucial step in modernizing health policy and decision-making. Although other models predict and analyze fine particulate matter exposure, they often rely on modeled input data sources and data streams that are not regularly updated. Another challenge stems from current models relying on predefined grids. In contrast, our deep-learning approach interpolates surface level PM2.5 concentrations between sparsely distributed US EPA monitoring stations in a grid-free manner. By incorporating additional, readily available datasets - including topographic, meteorological, and land-use data - we improve its ability to predict pollutant concentrations with high spatial and temporal resolution. This enables model querying at any spatial location for rapid predictions without computing over the entire grid. To ensure robustness, we randomize spatial sampling during training to enable our model to perform well in both dense and sparse monitored regions. This model is well suited for near real-time deployment because its lightweight architecture allows for fast updates in response to streaming data. Moreover, model flexibility and scalability allow it to be adapted to various geographical contexts and scales, making it a practical tool for delivering accurate and timely air quality assessments. Its capacity to rapidly evaluate multiple scenarios can be especially valuable for decision-making during public health crises.

Supervised learning with Earth observation inputs is often limited by the sparsity of high-quality labeled or in-situ measured data to use as training labels. With the abundance of geographic data products, in many cases there are variables correlated with - but different from - the variable of interest that can be leveraged. We integrate such proxy variables within a geographic prior via a trainable location encoder and introduce a proxy consistency loss (PCL) formulation to imbue proxy data into the location encoder. The first key insight behind our approach is to use the location encoder as an agile and flexible way to learn from abundantly available proxy data which can be sampled independently of training label availability. Our second key insight is that we will need to regularize the location encoder appropriately to achieve performance and robustness with limited labeled data. Our experiments on air quality prediction and poverty mapping show that integrating proxy data implicitly through the location encoder outperforms using both as input to an observation encoder and fusion strategies that use frozen, pretrained location embeddings as a geographic prior. Superior performance for in-sample prediction shows that the PCL can incorporate rich information from the proxies, and superior out-of-sample prediction shows that the learned latent embeddings help generalize to areas without training labels.